Multi-wave coherent control of a solid-state single emitter

Physical review letters, 2016

Coherent control of a strongly inhomogeneously broadened system, namely, InAs self-assembled quantum dots, is demonstrated. To circumvent the deleterious effects of the inhomogeneous broadening, which usually masks the results of coherent manipulation, we use prepulse two-dimensional coherent spectroscopy to provide a size-selective readout of the ground, exciton, and biexciton states. The dependence on the timing of the prepulse is due to the dynamics of the coherently generated populations. To further validate the results, we performed prepulse polarization dependent measurements and confirmed the behavior expected from selection rules. All measured spectra can be excellently reproduced by solving the optical Bloch equations for a 4-level system.

Japanese Journal of Applied Physics, 2004

We developed a high-resolution Michelson interferometer with a He-Ne two-frequency laser positioning system, and measured the coherent carrier dynamics of a single InAs self-assembled quantum dot (SAQD) using a micro-spectroscopy system. The phase-locked double pulses were stabilized, with the maximum deviation being below 10 nm during the long measurement time of 1 h. Using this system, coherent control of an exciton in an InAs SAQD with very fine phase stabilization was demonstrated. The dephasing time of the single quantum dots was 9.5 ps which is close to that estimated from the homogeneous linewidth in the photoluminescence excitation (PLE) spectrum.

Physical Review B, 2010

We demonstrate high-fidelity reversible transfer of quantum information from the polarisation of photons into the spin-state of an electron-hole pair in a semiconductor quantum dot. Moreover, spins are electrically manipulated on a sub-nanosecond timescale, allowing us to coherently control their evolution. By varying the area of the electrical pulse, we demonstrate phase-shift and spin-flip gate operations with near-unity fidelities. Our system constitutes a controllable quantum interface between flying and stationary qubits, an enabling technology for quantum logic in the solid-state.

Physical Review B, 2005

Using photoluminescence spectroscopy, we have investigated the nature of Rabi oscillation damping during optical manipulation of excitonic qubits in self-assembled quantum dots. Rabi oscillations were recorded by varying the pulse amplitude for fixed pulse durations between 4 ps and 10 ps. Up to five periods are visible, making it possible to quantify the excitation dependent damping. We find that this damping is more pronounced for shorter pulse widths and show that its origin is the nonresonant excitation of carriers in the wetting layer, most likely involving bound-to-continuum and continuum-to-bound transitions.

We propose an optoelectronic scheme to define and manipulate an indirect neutral exciton qubit within a quantum dot molecule. We demonstrate coherent dynamics of indirect excitons resilient against decoherence effects, including direct exciton spontaneous recombination. For molecules with large interdot separation, the exciton dressed spectrum yields an often overlooked avoided crossing between spatially indirect exciton states. Effective two-level system Hamiltonians are extracted by Feshbach projection over the multilevel exciton configurations. An adiabatic manipulation of the qubit states is devised using time-dependent electric field sweeps. The exciton dynamics yields the necessary conditions for qubit initialization and near unitary rotations in the picosecond time scale, driven by the system internal dynamics. Despite the strong influence of laser excitation, charge tunneling, and interdot dipole-dipole interactions, the effective relaxation time of indirect excitons is much longer than the direct exciton spontaneous recombination time, rendering indirect excitons as potential elemental qubits in more complex schemes.

In this work, we propose the use of the Hanbury-Brown and Twiss interferometric technique and a switchable two-color excitation method for evaluating the exciton and noncorrelated electron−hole dynamics associated with single photon emission from indium arsenide (InAs) selfassembled quantum dots (QDs). Using a microstate master equation model we demonstrate that our single QDs are described by nonlinear exciton dynamics. The simultaneous detection of two-color, single photon emission from InAs QDs using these nonlinear dynamics was used to design a NOT AND logic transference function. This computational functionality combines the advantages of working with light/photons as input/output device parameters (all-optical system) and that of a nanodevice (QD size of ∼20 nm) while also providing high optical sensitivity (ultralow optical power operational requirements). These system features represent an important and interesting step toward the development of new prototypes for the incoming quantum information technologies.

Physical Review B, 2013

Exciton, trion and biexciton dephasing rates are measured within the inhomogeneous distribution of an InAs quantum dot (QD) ensemble using two-dimensional Fourier-transform spectroscopy. The dephasing rate of each excitonic state is similar for all QDs in the ensemble and the rates are independent of excitation density. An additional spectral feature -too weak to be observed in the time-integrated four-wave mixing signal -appears at high excitation density and is attributed to the χ (5) biexcitonic nonlinear response.

Physical Review Letters, 2004

We report the first experimental study of the optical Stark effect in single semiconductor quantum dots (QD). For below band gap excitation, two-color pump-probe spectra show dispersive line shapes caused by a light-induced blueshift of the excitonic resonance. The line shape depends strongly on the excitation field strength and is determined by the pump-induced phase shift of the coherent QD polarization. Transient spectral oscillations can be understood as rotations of the QD polarization phase with negligible population change. Ultrafast control of the QD polarization is demonstrated.

Fast, controlled coherent interactions between spins in separated quantum dots are a key requirement for two-qubit gates and distributed architectures in advancing quantum information in the solid state. We have performed two-color pump-probe experiments in which pulsed lasers emitting at different photon energies manipulate two subsets of electron spins in an inhomogeneous ensemble of InGaAs quantum dots. Measurements of the resulting ellipticity demonstrate the slow, power dependent onset of phase shifts in the Larmor precession in a magnetic field of one subset of oriented spins after optical orientation of the second subset. Model calculations show that these results are consistent with a Heisenberg-like interaction between the pairs of spins with strength ~ µeV and that this interaction results in entanglement between the spins. Considerable progress has been made recently in establishing optical control of spins confined in semiconductor quantum dots, a system of interest as quantum bits (qubits) for implementations of quantum information (1). Single spin decoherence times on the order of microseconds have been demonstrated (2), and methods for spin initialization and

We propose a coherent control scheme based on the optical Stark effect in optically generated excitons in quantum dot molecules (QDMs). We show that, by the combined action of voltage bias detuning sweeps and Rosen-Zener pulsed interactions, it is possible to dynamically generate and modify an anticrossing gap that emerges between the dressed energy levels of long-lived, spatially indirect excitons. We perform numerical and analytic non-perturbative calculations based on the Bloch-Feshbach formalism, which demonstrate that this effect induces a mechanism of coherent population trapping of indirect excitons in QDMs. Our results show that it is possible to perform an all-optical implementation of indirect-excitonic qubit operations, such as the Pauli-X and Hadamard quantum gates, across two defined axis of the Bloch Sphere.